Estimated taxes may also include your refund from tax year 2020 and applied to your 2021 income tax return. To see if that is a 2020 amount carried over to your 2021 income tax return:
You could also take a look at your 1040 form. Preview your 1040. Look at line 26, 2021 estimated tax payments and amount applied form 2020 return to see if the $4,500 might be that.