If the LLC is earning money in PA, you would need to file a return in PA and Louisiana. You would file the PA return first, then you would take a credit on your Louisiana return for taxes paid to PA.
So, yes, you will be filing for both. Also, if you lived in PA for part of the year, you will be filing a Part Year resident return for both. PA you will include the income for the entire year. Louisiana, you will include the income you received while living in the state.
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