Yes, in fact you would create a new file for 2024 for both Federal and State, so that when you prepare PA, it will follow along with what you've done in the Federal, with you as the new primary taxpayer. You won't be able to use your old account if you are using TurboTax Online to do your Federal, then make changes to the primary taxpayer in the state. They'll have to be the same.
If you've already filed your Federal return, you can file your PA return through MyPath.
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