Item 104 on form 760 ADJ is for Virginia 529 contributions, which are not charitable contributions. Where do you see that 104 refers to charitable contributions?
106 indeed refers to long term care premiums. You can deduct the long-term care premiums provided that you did not enter these on the federal and itemized (i.e., derived a benefit on the federal return from the premiums).
In the Virginia interview, there is a screen "Here's the income that Virginia handles differently". Scroll down to Medical and click on Start for Long-term Care Premiums Deduction.
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