Yes, you still must submit IT-2105.9 with your NY IT-201 for 2021.
Per the IT-210.9 instructions, you may be charged a penalty if you did not pay enough estimated tax by any of the due dates or if you did not have enough New York State, New York City, or Yonkers income tax withheld. Although you will be paying the underpayment by 4/15/2022 (the due date of the return), you may owe the penalty for an earlier payment due date, even if you paid enough tax later to make up the underpayment.
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